Advanced Search+
Pan CHEN (陈攀), Jun SHEN (沈俊), Tangchun RAN (冉唐春), Tao YANG (杨涛), Yongxiang YIN (印永祥). Investigation of operating parameters on CO2 splitting by dielectric barrier discharge plasma[J]. Plasma Science and Technology, 2017, 19(12): 125505. DOI: 10.1088/2058-6272/aa8903
Citation: Pan CHEN (陈攀), Jun SHEN (沈俊), Tangchun RAN (冉唐春), Tao YANG (杨涛), Yongxiang YIN (印永祥). Investigation of operating parameters on CO2 splitting by dielectric barrier discharge plasma[J]. Plasma Science and Technology, 2017, 19(12): 125505. DOI: 10.1088/2058-6272/aa8903

Investigation of operating parameters on CO2 splitting by dielectric barrier discharge plasma

Funds: The authors gratefully acknowledge the support of National Natural Science Foundation of China (No. 11375123).
More Information
  • Received Date: February 20, 2017
  • Experiments of CO2 splitting by dielectric barrier discharge (DBD) plasma were carried out, and the influence of CO2 flow rate, plasma power, discharge voltage, discharge frequency on CO2 conversion and process energy efficiency were investigated. It was shown that the absolute quantity of CO2 decomposed was only proportional to the amount of conductive electrons across the discharge gap, and the electron amount was proportional to the discharge power; the energy efficiency of CO2 conversion was almost a constant at a lower level, which was limited by CO2 inherent discharge character that determined a constant gap electric field strength. This was the main reason why CO2 conversion rate decreased as the CO2 flow rate increase and process energy efficiency was decreased a little as applied frequency increased. Therefore, one can improve the CO2 conversion by less feed flow rate or larger discharge power in DBD plasma, but the energy efficiency is difficult to improve.
  • [1]
    Gurney K R et al 2009 Environ. Sci. Technol. 43 5535
    [2]
    Pardia B, Iniyan S and Goic R 2011 Renew. Sustain. Energy Rev. 15 1625
    [3]
    Thirugnanasambandam M, Iniyan S and Goic R 2010 Renew. Sustain. Energy Rev. 14 312
    [4]
    Lebouvier A et al 2013 Energy Fuels 27 2712
    [5]
    Li D H et al 2009 Int. J. Hydrogen Energy 34 308
    [6]
    Tomishige K, Chen Y G and Fujimoto K 1999 J. Catal. 181 91
    [7]
    Zhang Y P et al 2016 Chem. J. Chin. Univ. 37 1521 (in Chinese)
    [8]
    Zeng W X and Tu X 2017 J. Phys. D: Appl. Phys. 50 184004
    [9]
    Moss M S et al 2017 Plasma Sources Sci. Technol. 26 035009
    [10]
    Horváth G et al 2008 J. Phys. D: Appl. Phys. 41 225207
    [11]
    Kim S C and Chun Y N 2014 Environ. Technol. 35 2940
    [12]
    Heijkers S et al 2015 J. Phys. Chem. C 119 12815
    [13]
    Aerts R, Somers W and Bogaerts A 2015 ChemSusChem 8 702
    [14]
    Ponduri S et al 2016 J. Appl. Phys. 119 093301
    [15]
    Kogelschatz U 2003 Plasma Chem. Plasma Process. 23 1
    [16]
    Ozkan A, Bogaerts A and Reniers F 2017 J. Phys. D: Appl. Phys. 50 084004
    [17]
    Paulussen S et al 2010 Plasma Sources Sci. Technol. 19 034015
    [18]
    Brehmer F et al 2014 J. Appl. Phys. 116 123303
    [19]
    Aerts R, Martens T and Bogaerts A 2012 J. Phys. Chem. C 116 23257
    [20]
    Ozkan A et al 2016 Plasma Sources Sci. Technol. 25 025013
    [21]
    Manley T C 1943 J. Electrochem. Soc. 84 83
    [22]
    Valdivia-Barrientos R et al 2006 Plasma Sources Sci. Technol. 15 237
    [23]
    Fridman A 2008 Plasma Chemistry (London: Cambridge University Press)
    [24]
    Mei D H et al 2015 Plasma Sources Sci. Technol. 24 015011
    [25]
    Yu Q Q et al 2012 Plasma Chem. Plasma Process. 32 153
    [26]
    Ramakers M et al 2015 Plasma Process. Polym. 12 755
  • Related Articles

    [1]David BAILIE, Cormac HYLAND, Raj L SINGH, Steven WHITE, Gianluca SARRI, Francis P KEENAN, David RILEY, Steven J ROSE, Edward G HILL, Feilu WANG (王菲鹿), Dawei YUAN (袁大伟), Gang ZHAO (赵刚), Huigang WEI (魏会冈), Bo HAN (韩波), Baoqiang ZHU (朱宝强), Jianqiang ZHU (朱健强), Pengqian YANG (杨朋千). An investigation of the L-shell x-ray conversion efficiency for laser-irradiated tin foils[J]. Plasma Science and Technology, 2020, 22(4): 45201-045201. DOI: 10.1088/2058-6272/ab6188
    [2]Peng LIU (刘朋), Xuesong LIU (刘雪松), Jun SHEN (沈俊), Yongxiang YIN (印永祥), Tao YANG (杨涛), Qiang HUANG (黄强), Daniel AUERBACH, Aart W KLEIYN. CO2 conversion by thermal plasma with carbon as reducing agent: high CO yield and energy efficiency[J]. Plasma Science and Technology, 2019, 21(1): 12001-012001. DOI: 10.1088/2058-6272/aadf30
    [3]Dan ZHAO (赵丹), Feng YU (于锋), Amin ZHOU (周阿敏), Cunhua MA (马存花), Bin DAI (代斌). High-efficiency removal of NOx using dielectric barrier discharge nonthermal plasma with water as an outer electrode[J]. Plasma Science and Technology, 2018, 20(1): 14020-014020. DOI: 10.1088/2058-6272/aa861c
    [4]Yunfeng HAN (韩云峰), Shaoyang WEN (温少扬), Hongwei TANG (汤红卫), Xianhu WANG (王贤湖), Chongshan ZHONG (仲崇山). Influences of frequency on nitrogen fixation of dielectric barrier discharge in air[J]. Plasma Science and Technology, 2018, 20(1): 14001-014001. DOI: 10.1088/2058-6272/aa947a
    [5]Xu CAO (曹栩), Weixuan ZHAO (赵玮璇), Renxi ZHANG (张仁熙), Huiqi HOU (侯惠奇), Shanping CHEN (陈善平), Ruina ZHANG (张瑞娜). Conversion of NO with a catalytic packed-bed dielectric barrier discharge reactor[J]. Plasma Science and Technology, 2017, 19(11): 115504. DOI: 10.1088/2058-6272/aa7ced
    [6]N KHADIR, K KHODJA, A BELASRI. Methane conversion using a dielectric barrier discharge reactor at atmospheric pressure for hydrogen production[J]. Plasma Science and Technology, 2017, 19(9): 95502-095502. DOI: 10.1088/2058-6272/aa6d6d
    [7]Mook Tzeng LIM (林木森), Ahmad Zulazlan SHAH ZULKIFLI, Kanesh Kumar JAYAPALAN, Oihoong CHIN. Development of a dimensionless parameter for characterization of dielectric barrier discharge devices with respect to geometrical features[J]. Plasma Science and Technology, 2017, 19(9): 95402-095402. DOI: 10.1088/2058-6272/aa7382
    [8]YAO Shuiliang (姚水良), WENG Shan (翁珊), JIN Qi (金旗), HAN Jingyi (韩竞一), JIANG Boqiong (江博琼), WU Zuliang (吴祖良). Equation of Energy Injection to a Dielectric Barrier Discharge Reactor[J]. Plasma Science and Technology, 2016, 18(8): 804-811. DOI: 10.1088/1009-0630/18/8/03
    [9]SUN Hao (孙昊), WU Yi (吴翊), RONG Mingzhe (荣命哲), GUO Anxiang (郭安祥), HAN Guiquan (韩桂全), LU Yanhui (卢彦辉). Investigation on the Dielectric Properties of CO2 and CO2-Based Gases Based on the Boltzmann Equation Analysis[J]. Plasma Science and Technology, 2016, 18(3): 217-222. DOI: 10.1088/1009-0630/18/3/01
    [10]ZHANG Ying(张颖), LI Jie(李杰), LU Na(鲁娜), SHANG Kefeng(商克峰), WU Yan(吴彦). Diagnosis of Electronic Excitation Temperature in Surface Dielectric Barrier Discharge Plasmas at Atmospheric Pressure[J]. Plasma Science and Technology, 2014, 16(2): 123-127. DOI: 10.1088/1009-0630/16/2/07

Catalog

    Article views (210) PDF downloads (596) Cited by()

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return