Decomposition of a gas mixture of four n-alkanes using a DBD reactor

Boqiong JIANG (江博琼); Xiaodan FEI (费小丹); Shuiliang YAO (姚水良); Qinmin WANG (王钦民); Xinlei YAO (姚馨蕾); Kai XU (徐锴); Zhizong CHEN (陈挚宗)

doi:10.1088/2058-6272/aba2c3

Plasma Science and Technology > 2020 > 22(11): 115501. > DOI: 10.1088/2058-6272/aba2c3

Boqiong JIANG (江博琼), Xiaodan FEI (费小丹), Shuiliang YAO (姚水良), Qinmin WANG (王钦民), Xinlei YAO (姚馨蕾), Kai XU (徐锴), Zhizong CHEN (陈挚宗). Decomposition of a gas mixture of four n-alkanes using a DBD reactor[J]. Plasma Science and Technology, 2020, 22(11): 115501. DOI: 10.1088/2058-6272/aba2c3

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Decomposition of a gas mixture of four n-alkanes using a DBD reactor

¹ School of Environmental Science and Engineering, Zhejiang Gongshang University, Hangzhou 310018, People's Republic of China
² School of Environmental and Safety Engineering, Changzhou University, Changzhou 213164, People's Republic of China

Funds: This work was supported by the Zhejiang Basic Public Welfare Research Program (No. LGG19E080001) and Natural Science Foundation of Zhejiang Province (No. LY19B070002).

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Received Date: March 31, 2020
Revised Date: July 01, 2020
Accepted Date: July 02, 2020

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Abstract

Abstract

This study investigates the decomposition of a gas mixture of four n-alkanes (n-heptane, n-octane, n-nonane, and n-decane) using a dielectric barrier discharge reactor. We show that the conversion of n-alkanes increased from 7.2% (C₇H₁₆), 9.7% (C₈H₁₈), 8.4% (C₉H₂₀), and 10.5% (C₁₀H₂₂) to 23.8% (C₇H₁₆), 25.0% (C₈H₁₈), 27.9% (C₉H₂₀), and 32.1% (C₁₀H₂₂) when the energy density increased from 84 J l⁻¹ to 324 J l⁻¹. The conversion of n-alkanes when using the gas mixture is close to that found when using a single n-alkane. The influences of reaction temperature and O₂ concentration are also investigated, and the activation energies for the decomposition of each alkane are given.
- multiple components,
- n-alkane decomposition,
- dielectric barrier discharge,
- energyefficiency,
- activation energy

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References

[1]	Hui L R et al 2020 Atmos. Environ. 224 117340
[2]	Chen G B et al 2018 Environ. Int. 121 1121
[3]	Chaichan M T and Abass Q A 2010 Al-Khwarizmi Eng. J. 6 11
[4]	Vo T D H et al 2018 J. Environ. Manage. 217 327
[5]	Liu Y et al 2017 DEStech transactions on engineering and technology research Proc. 2017 4th Int. Conf. on Engineering Technology and Application (ICAENM 2017) (Nagoya, Japan) (DEStech Publications) 2017
[6]	Hanna S R et al 2007 J. Appl. Meteor. Climatol. 46 1372
[7]	Boeglin M L, Wessels D and Henshel D 2006 Environ. Res.100 242
[8]	Sousa S I V, Alvim-Ferraz M C M and Martins F G 2013 Chemosphere 90 2051
[9]	Cai C J et al 2010 Atmos. Environ. 44 5005
[10]	An J L et al 2014 Atmos. Environ. 97 206
[11]	Li Q Q et al 2020 Sci. Total Environ. 720 137536
[12]	Özbuğday F C and Erbas B C 2015 Energy 82 734
[13]	Ghoreyshi A A, Sadeghifar H and Entezarion F 2014 Energy 73 838
[14]	Hu J et al 2016 Chem. Eng. J. 293 216
[15]	Kado S et al 2003 Fuel 82 1377
[16]	Najafpoor A A et al 2018 Environ. Sci. Pollut. Res. 25 233
[17]	Karuppiah J et al 2012 J. Hazard. Mater. 237–238 283
[18]	Jiang N et al 2016 IEEE Trans. Plasma Sci. 44 657
[19]	Sekiguchi H 2001 Can. J. Chem. Eng. 79 512
[20]	Subrahmanyam C, Renken A and Kiwi-Minsker L 2006 Appl.Catal. B 65 157
[21]	Ma T P et al 2016 Plasma Chem. Plasma Process. 36 1533
[22]	Karatum O and Deshusses M A 2016 Chem. Eng. J. 294 308
[23]	Jiang L Y et al 2017 J. Environ. Sci. 55 266
[24]	Zhu R Y et al 2015 Chem. Eng. J. 279 463
[25]	Ding H X et al 2006 J. Phys. D Appl. Phys. 39 3603
[26]	Chang M B and Lee H M 2004 Catal. Today 89 109
[27]	Jin Q et al 2016 Chem. Eng. J. 286 300
[28]	Jin Q 2015 Study on n-alkane decomposition using dielectric barrier discharges MSc Thesis Zhejiang Gongshang University (in Chinese)
[29]	Rousso A et al 2019 Proc. Combust. Inst. 37 5595
[30]	Yao S L, Zhang X M and Lu H 2020 High Voltage Eng. 46 342 (in Chinese)
[31]	Wang R C et al 2020 J. Environ. Sci. 96 138
[32]	Dean J A 1985 Lang’s Handbook of Chemistry 13th edn (New York: McGraw-Hill)
[33]	Kitayama J and Kuzumoto M 1999 J. Phys. D Appl. Phys.32 3032
[34]	Tang Q et al 2011 Ind. Eng. Chem. Res. 50 9839
[35]	Penetrante B M et al 1997 Plasma Sources Sci. Technol. 6 251
[36]	Jiang N et al 2013 J. Hazard. Mater. 262 387
[37]	Liang W J et al 2015 J. Electrost. 75 27
[38]	Yao S L et al 2016 IEEE Trans. Plasma Sci. 44 2660
[39]	Vandenbroucke A M et al 2011 J. Hazard. Mater. 195 30
[40]	Battin-Leclerc F 2008 Prog. Energy Combust. Sci. 34 440
[41]	Xu W and Fan H J 2018 Fuel 234 1165
[42]	Marotta E and Paradisi C 2009 J. Am. Soc. Mass Spectrom.20 697
[43]	Yao S L et al 2015 J. Electrost. 75

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Decomposition of a gas mixture of four n-alkanes using a DBD reactor