Numerical investigation on electron effects in the mass transfer of the plasma species in aqueous solution

Xiaolong WANG (王晓龙); Zhenyu TAN (谭震宇); Jiaqi HAN (韩佳奇); Xiaotong LI (李晓彤)

doi:10.1088/2058-6272/abaaa4

Plasma Science and Technology > 2020 > 22(11): 115504. > DOI: 10.1088/2058-6272/abaaa4

Xiaolong WANG (王晓龙), Zhenyu TAN (谭震宇), Jiaqi HAN (韩佳奇), Xiaotong LI (李晓彤). Numerical investigation on electron effects in the mass transfer of the plasma species in aqueous solution[J]. Plasma Science and Technology, 2020, 22(11): 115504. DOI: 10.1088/2058-6272/abaaa4

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Numerical investigation on electron effects in the mass transfer of the plasma species in aqueous solution

School of Electrical Engineering, Shandong University, Jinan 250061, People's Republic of China

Funds: This work was supported by the Fundamental Research Funds of Shandong University (2018TB037).

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Received Date: May 11, 2020
Revised Date: July 27, 2020
Accepted Date: July 28, 2020

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Abstract

Abstract

The objective of this work is to contribute an understanding of the effects of electrons in the plasmas on the mass transfer of plasma species in aqueous solution by means of the numerical simulation based on a one-dimensional diffusion-reaction model. The plasma species are divided into two groups, i.e. electrons and the other species, and the mass transfer in the three scenarios has been simulated, including the systematic calculations of the depth distributions of five major reactive species, OH, O₃, HO₂, O₂^-, and H₂O₂ . In the three scenarios, the particles considered to enter into aqueous solution are all the plasma species (the scenario I, where the mass transfer of plasma species is a result due to the synergy of the electrons and the other plasma species), the other species (the scenario II), and only electrons in plasma species (the scenario III), respectively. The detailed analyses on the difference between the depth distributions of each reactive species in these three scenarios show the following conclusions. The electrons play an important role in the mass transfer of plasma species in aqueous solution and the synergy of the electrons and the other plasma species (the electron-species synergy) presents its different effects on the mass transfer. The vast majority of H₂O₂ are generated from a series of the electron- related reactions in aqueous solution, which is hardly affected by the electron-species synergy. Compared to the results when only the electrons enter into the liquid region, the electron-species synergy evidently weakens the generation of O₂^-, O₃, and OH, but promotes to produce HO₂ .
- plasma species,
- electron effect,
- mass transfer,
- aqueous solution,
- plasma biomedicine

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References

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Numerical investigation on electron effects in the mass transfer of the plasma species in aqueous solution