Study of tetracycline removal and saturated resin regenerated by dielectric barrier discharge plasma

Chunjing HAO (郝春静); Zeyao YAN (闫泽垚); Kefu LIU (刘克富); Jian QIU (邱剑)

doi:10.1088/2058-6272/ac2225

Plasma Science and Technology > 2021 > 23(11): 115506. > DOI: 10.1088/2058-6272/ac2225

Chunjing HAO (郝春静), Zeyao YAN (闫泽垚), Kefu LIU (刘克富), Jian QIU (邱剑). Study of tetracycline removal and saturated resin regenerated by dielectric barrier discharge plasma[J]. Plasma Science and Technology, 2021, 23(11): 115506. DOI: 10.1088/2058-6272/ac2225

Citation:

PDF (1926 KB)

Study of tetracycline removal and saturated resin regenerated by dielectric barrier discharge plasma

School of Information Science and Technology, Department of Light Sources & Illuminating Engineering, Fudan University, Shanghai 200433, People's Republic of China

Funds: This research has been financed by National Natural Science Foundation of China (No. 51877046). The financial support is gratefully acknowledged.

More Information

Received Date: June 21, 2021
Revised Date: August 24, 2021
Accepted Date: August 26, 2021

Graphical Abstract

Abstract

Abstract

The wastewater produced by the large-scale usage of antibiotics worldwide was more harmful to the ecological environment and human health. In the research, the coupling technology of ‘adsorption-plasma regeneration’ was taken to treat tetracycline in aqueous solution. The pollutants were adsorbed by the resins firstly and then regenerated ectopically by dielectric barrier discharge plasma. The discharge parameters, such as discharge voltage and frequency were researched to achieve the optimal regeneration efficiency and energy efficiency. Meanwhile, the analyses of the surface functional groups and microstructure were also investigated. After the five ‘adsorption-regeneration’ processes, the results showed that the optimal discharge parameters of voltage and frequency were 20 kV and 1 kHz, respectively. The regeneration efficiency and energy efficiency were above 80% and 115 g kW⁻¹ ·h⁻¹, respectively. The tetracycline adsorption by virgin resin and regenerated resin nearly followed pseudo-second order kinetics, and there was no fatal damage to the surface characteristics and physicochemical properties of the resins through the multiple plasma regeneration processes. Finally, according to the intra-particle diffusion model and the degradation products detected by GC-MS, the adsorption and degradation mechanisms of tetracycline were deduced.
- adsorbtion,
- regeneration,
- tetracycline,
- resin,
- DBD plasma,
- mechanism

FullText(HTML)

References (35)

References

[1]	Heddini A et al 2009 Lancet 373 30
[2]	Schübler M 2009 CLEAN—Soil Air Water 37 514
[3]	Daghrir R and Drogui P 2013 Environ. Chem. Lett. 11 209
[4]	Hou J et al 2016 Environ. Sci. Pollut. Res. 23 1722
[5]	Phoon B L et al 2020 J. Hazard. Mater. 400 122961
[6]	Abejón R et al 2015 Water Res. 73 118
[7]	Dong H Y et al 2016 J. Environ. Manage. 178 11
[8]	Xiang L R et al 2021 Chemosphere 283 131156
[9]	Samukawa S et al 2012 J. Phys. D: Appl. Phys. 45 253001
[10]	Guo H et al 2018 Vacuum 156 402
[11]	Kogelschatz U 2003 Plasma Chem. Plasma Process. 23 1
[12]	Locke B R and Shih K Y 2011 Plasma Sources Sci. Technol.20 034006
[13]	Lu B et al 2008 J. Mater. Eng. Perform. 17 428
[14]	Yamamoto Y, Yang C L and Zhang R H 1998 New emission control using nonthermal plasma desorption Proc. 91st Annual Meeting & Exhibition of Air & Waste Management Association (San Diego)
[15]	Quan X et al 2004 Water Res. 38 4484
[16]	Gaffney J S, Marley N A and Jones D E 2009 Fourier Transform Infrared (FTIR) Spectroscopy: Infrared Spectroscopy for Food Quality Analysis and Control (New York: Wiley)
[17]	Zhao Y P et al 2012 Geoderma 183–184 12
[18]	de Sousa F B et al 2008 Vib. Spectrosc. 46 57
[19]	Weber W J Jr et al 1963 J. Sanit. Eng. Div. Am. Soc. Civil Eng.89 31
[20]	Hu X J et al 2017 Int. J. Environ. Res. Public Health 14 1495
[21]	Behera S K et al 2011 Sci. Total Environ. 409 4351
[22]	Chen B et al 2015 Environ. Sci. Pollut. Res. 22 13950
[23]	Herzberg 1983 Molecular Spectroscopy and Molecular Structure (Beijing: Science Press) (in Chinese)
[24]	Pietsch G J and Gibalov V I 1998 Pure Appl. Chem. 70 1169
[25]	Samaranayake W J M et al 2000 IEEE Trans. Dielectr. Electr.Insul. 7 849
[26]	Chen Y M et al 2004 J. Electr. Devices 27 653 (in Chinese)
[27]	Xu G H 2006 Plasma Technology and Application (Beijing:Chemical Industry Press) (in Chinese)
[28]	Tas M A 1995 Plasma-induced catalysis: a feasibility study and fundamentals PhD Thesis Technische Universiteit Eindhoven
[29]	Yao W L et al 2010 Environ. Sci. Res. 1 1192 (in Chinese)
[30]	Fincke J R et al 2002 Plasma Chem. Plasma Process. 22 105
[31]	Jiang T et al 2002 Catal. Today 72 229
[32]	Zhou L M et al 1998 Plasma Chem. Plasma Process. 18 375
[33]	Chen L et al 2009 Chem. Eng. Process.: Process Intensif.48 1333
[34]	Leidner D et al 1991 Organic Chemistry of Drug Synthesis (Beijing: Chemical Industry Press) (in Chinese)
[35]	Dmuchovsky B et al 1965 J. Catal. 4 291

[1]	Tianchi WANG, Chuyu SUN, Youheng YANG, Haiyang WANG, Linshen XIE, Tao HUANG, Yingchao DU, Wei CHEN. Comparative study of pulsed breakdown processes and mechanisms in self-triggered four-electrode pre-ionized switches[J]. Plasma Science and Technology, 2022, 24(11): 115504. DOI: 10.1088/2058-6272/ac7c61
[2]	Tianchi WANG (王天驰), Yingchao DU (杜应超), Wei CHEN (陈伟), Junna LI (李俊娜), Haiyang WANG (王海洋), Tao HUANG (黄涛), Linshen XIE (谢霖燊), Le CHENG (程乐), Ling SHI (石凌). A low-jitter self-triggered spark-discharge pre-ionization switch: primary research on its breakdown characteristics and working mechanisms[J]. Plasma Science and Technology, 2021, 23(11): 115508. DOI: 10.1088/2058-6272/ac2420
[3]	Rongxiao ZHAI (翟戎骁), Tao HUANG (黄涛), Peitian CONG (丛培天), Weixi LUO (罗维熙), Zhiguo WANG (王志国), Tianyang ZHANG (张天洋), Jiahui YIN (尹佳辉). Comparative study on breakdown characteristics of trigger gap and overvoltage gap in a gas pressurized closing switch[J]. Plasma Science and Technology, 2019, 21(1): 15505-015505. DOI: 10.1088/2058-6272/aae432
[4]	Xifeng CAO (曹希峰), Guanrong HANG (杭观荣), Hui LIU (刘辉), Yingchao MENG (孟颖超), Xiaoming LUO (罗晓明), Daren YU (于达仁). Hybrid–PIC simulation of sputtering product distribution in a Hall thruster[J]. Plasma Science and Technology, 2017, 19(10): 105501. DOI: 10.1088/2058-6272/aa7940
[5]	JIAO Zhihong (焦志宏), WANG Guoli (王国利), ZHOU Xiaoxin (周效信), WU Chaohui (吴朝辉), ZUO Yanlei (左言磊), ZENG Xiaoming (曾小明), ZHOU Kainan (周凯南), SU Jingqin (粟敬钦). Study on the Two-Dimensional Density Distribution for Gas Plasmas Driven by Laser Pulse[J]. Plasma Science and Technology, 2016, 18(12): 1169-1174. DOI: 10.1088/1009-0630/18/12/05
[6]	CHENG Anyi (成安义), ZHANG Qiyong (张启勇), FU Bao (付豹), LU Xiaofei (陆小飞). Process Design of Cryogenic Distribution System for CFETR CS Model Coil[J]. Plasma Science and Technology, 2016, 18(2): 202-205. DOI: 10.1088/1009-0630/18/2/18
[7]	WU Xingquan (伍兴权), LUO Jiarong (罗家融), WU Bin (吴斌), WANG Jinfang (王进芳), HU Chundong (胡纯栋). Calculation of Shinethrough and its Power Density Distribution for EAST NBI[J]. Plasma Science and Technology, 2013, 15(5): 480-484. DOI: 10.1088/1009-0630/15/5/17
[8]	LI Shuang(李双), FENG Shengqin (冯笙琴). Gluon Saturation Model with Geometric Scaling for Net-Baryon Distributions in Relativistic Heavy Ion Collisions[J]. Plasma Science and Technology, 2012, 14(7): 598-602. DOI: 10.1088/1009-0630/14/7/07
[9]	LIU Peng (刘鹏), SUN Fengju (孙凤举), WEI Hao (魏浩), Wang Zhiguo (王志国), YIN Jiahui (尹佳辉), QIU Aici (邱爱慈). Influences of Switching Jitter on the Operational Performances of Linear Transformer Drivers -Based Drivers[J]. Plasma Science and Technology, 2012, 14(4): 347-352. DOI: 10.1088/1009-0630/14/4/15
[10]	ZHU Ximing (朱悉铭), PU Yikang (蒲以康). Determination of Non-Maxwellian Electron Energy Distributions in Low-Pressure Plasmas by Using the Optical Emission Spectroscopy and a Collisional-Radiative Model[J]. Plasma Science and Technology, 2011, 13(3): 267-278.

Cited By

Cited by

Periodical cited type(6)

1.	Wang, T., Du, Y., Chen, W. A Review on Megavolt Pulsed Switches and Their Time Delay Jitters. IEEE Transactions on Plasma Science, 2024. DOI:10.1109/TPS.2024.3477737
2.	Wang, T., Sun, C., Yang, Y. et al. Comparative study of pulsed breakdown processes and mechanisms in self-triggered four-electrode pre-ionized switches. Plasma Science and Technology, 2022, 24(11): 115504. DOI:10.1088/2058-6272/ac7c61
3.	Wang, T., Wang, H., Huang, T. et al. Influence factors of the pulsed breakdown time delay jitter of a self-triggered UV-illuminated switch and an improvement method \| [自触发紫外预电离开关脉冲击穿时延抖动影响因素及改进方法]. Qiangjiguang Yu Lizishu/High Power Laser and Particle Beams, 2022, 34(7): 075010. DOI:10.11884/HPLPB202234.210459
4.	Wang, T., Li, J., Wang, H. et al. Optical Diagnosis of Preionization Mechanisms and Breakdown Characteristics in a Nanosecond Switch. IEEE Transactions on Plasma Science, 2022, 50(6): 1912-1926. DOI:10.1109/TPS.2022.3173423
5.	Wang, T., Huang, T., Wang, H. et al. Using Self-Triggered Sustaining Pre-Ionization to Obtain Nanosecond Jitter in a MV Pulsed Gas Switch. IEEE Transactions on Plasma Science, 2021, 49(12): 4034-4037. DOI:10.1109/TPS.2021.3127946
6.	Wang, T., Du, Y., Chen, W. et al. A low-jitter self-triggered spark-discharge pre-ionization switch: Primary research on its breakdown characteristics and working mechanisms. Plasma Science and Technology, 2021, 23(11): 115508. DOI:10.1088/2058-6272/ac2420

Other cited types(0)

Get Citation

PDF

XML

Article views (130) PDF downloads (67) Cited by(6)

Turn off MathJax

Article Contents

Abstract

References

Study of tetracycline removal and saturated resin regenerated by dielectric barrier discharge plasma