Insight into the remaining high surface energy of atmospheric DBD plasma-treated polyethylene web after three months’ aging

Hua LI (李花); Zhengduo WANG (王正铎); Lizhen YANG (杨丽珍); Qiang CHEN (陈强)

doi:10.1088/2058-6272/aae2ad

Plasma Science and Technology > 2019 > 21(1): 15504-015504. > DOI: 10.1088/2058-6272/aae2ad

Hua LI (李花), Zhengduo WANG (王正铎), Lizhen YANG (杨丽珍), Qiang CHEN (陈强). Insight into the remaining high surface energy of atmospheric DBD plasma-treated polyethylene web after three months’ aging[J]. Plasma Science and Technology, 2019, 21(1): 15504-015504. DOI: 10.1088/2058-6272/aae2ad

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Insight into the remaining high surface energy of atmospheric DBD plasma-treated polyethylene web after three months’ aging

Laboratory of Plasma Physics & Materials, Beijing Institute of Graphic Communication, Beijing 102600, People’s Republic of China

Funds: Supported by National Natural Science Foundation of China (Nos. 11775028, 11505013), Beijing Municipal National Science Foundation (Nos. 4162024, KM201510015009), and the Collaborative Innovation Center of Green Printing & Publishing Technology (No. 20160113).

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Received Date: August 02, 2018

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Abstract

In this paper, we report the modification of polyethylene (45 μm in thickness) webs through a roll-to-roll dielectric barrier discharge plasma treatment in an open atmospheric environment. Our work differs from the normal adopted corona discharge treatment at an atmospheric pressure, in that three monomers: allylamine, acrylic acid, and ethanol, are inlet into the discharge zone by argon (Ar) carrier gas. As a comparison, Ar plasma treatment is also carried out. We focus on the aging properties of treated plastics in the open air. It is found that the modified webs can retain the surface energy as high as 50.0±1 mN m^-1 for more than three months. After characterization of the as-prepared and aged samples by the surface roughness, the wettability, and the chemical structure, the mechanism of retaining high surface energy is then presumed. We think that the initial high surface energy just after plasma treatment is correlated to the grafted functional groups, while the over 50.0 mN m^-1 remaining surface energy after three month aging is due to the stable concentrations of oxygen-contained and nitrogen-contained groups by post-reaction on the surfaces.
- aging,
- atmospheric DBD treatment,
- polyethylene,
- surface energy remaining

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References

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Insight into the remaining high surface energy of atmospheric DBD plasma-treated polyethylene web after three months’ aging