Enhanced CO<sub>2</sub> decomposition via metallic foamed electrode packed in self-cooling DBD plasma device

Shengjie ZHU (朱圣洁); Amin ZHOU (周阿敏); Feng YU (于锋); Bin DAI (代斌); Cunhua MA (马存花)

doi:10.1088/2058-6272/ab15e5

Plasma Science and Technology > 2019 > 21(8): 85504-085504. > DOI: 10.1088/2058-6272/ab15e5

Shengjie ZHU (朱圣洁), Amin ZHOU (周阿敏), Feng YU (于锋), Bin DAI (代斌), Cunhua MA (马存花). Enhanced CO₂ decomposition via metallic foamed electrode packed in self-cooling DBD plasma device[J]. Plasma Science and Technology, 2019, 21(8): 85504-085504. DOI: 10.1088/2058-6272/ab15e5

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Enhanced CO₂ decomposition via metallic foamed electrode packed in self-cooling DBD plasma device

¹ School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, People’s Republic of China
² Laboratory of Plasma Physical Chemistry, Dalian University of Technology, Dalian 116024, People’s Republic of China

Funds: This work was financially supported by the National Natural Science Foundation of China (No. 21663022).

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Received Date: December 23, 2018
Revised Date: April 01, 2019
Accepted Date: April 03, 2019

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Abstract

Abstract

A self-cooling dielectric barrier discharge reactor, packed with foamed Cu and Ni mesh and operated at ambient conditions, was used for the composition of CO₂ into CO and O₂. The influences of power, frequency, and other discharge characteristics were investigated in order to have a better understanding of the effect of the packing materials on CO₂ decomposition. It is found that porous foamed Cu and Ni not only played a role as the carrier of energy transformation and electrode distributed in discharge gaps but also promoted the equilibrium shifting toward the product side to yield more CO by consuming some part of O₂ and O radicals generated from the decomposition of CO₂. The maximum CO₂ decomposition rates of 48.6% and 49.2% and the maximum energy efficiency of 9.71% and 10.18% were obtained in the foamed Ni and Cu mesh, respectively.
- dielectric barrier discharge,
- CO₂ decomposition,
- metallic foamed materials,
- energy efficiency

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Enhanced CO₂ decomposition via metallic foamed electrode packed in self-cooling DBD plasma device

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Enhanced CO₂ decomposition via metallic foamed electrode packed in self-cooling DBD plasma device