The structure optimization of gas-phase surface discharge and its application for dye degradation

Ying CAO (曹颖); Jie LI (李杰); Nan JIANG (姜楠); Yan WU (吴彦); Kefeng SHANG (商克峰); Na LU (鲁娜)

doi:10.1088/2058-6272/aaa3d5

Plasma Science and Technology > 2018 > 20(5): 54018-054018. > DOI: 10.1088/2058-6272/aaa3d5

Ying CAO (曹颖), Jie LI (李杰), Nan JIANG (姜楠), Yan WU (吴彦), Kefeng SHANG (商克峰), Na LU (鲁娜). The structure optimization of gas-phase surface discharge and its application for dye degradation[J]. Plasma Science and Technology, 2018, 20(5): 54018-054018. DOI: 10.1088/2058-6272/aaa3d5

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The structure optimization of gas-phase surface discharge and its application for dye degradation

1 School of Environmental Science & Technology, Dalian University of Technology, Dalian 116023, People’s Republic of China 2 School of Electrical Engineering, Dalian University of Technology, Dalian 116024, People’s Republic of China

Funds: The authors would like to thank National Natural Science Foundation of China (No. 51477025)

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Received Date: October 30, 2017

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Abstract

Abstract

A gas-phase surface discharge (GSD) was employed to optimize the discharge reactor structure and investigate the dye degradation. A dye mixture of methylene blue, acid orange and methyl orange was used as a model pollutant. The results indicated that the reactor structure of the GSD system with the ratio of tube inner surface area and volume of 2.48, screw pitch between a high-voltage electrode of 9.7 mm, high-voltage electrode wire diameter of 0.8 mm, dielectric tube thickness of 2.0 mm and tube inner diameter of 16.13 mm presented a better ozone (O₃) generation efficiency. Furthermore, a larger screw pitch and smaller wire diameter enhanced the O₃ generation. After the dye mixture degradation by the optimized GSD system, 73.21% and 50.74% of the chemical oxygen demand (COD) and total organic carbon removal rate were achieved within 20 min, respectively, and the biochemical oxygen demand (BOD) and biodegradability (BOD/COD) improved.
- gas-phase surface discharge (GSD),
- structure optimization,
- ozone (O₃),,
- dye,
- degradation

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The structure optimization of gas-phase surface discharge and its application for dye degradation