Naphthalene oxidation by different non-thermal electrical discharges at atmospheric pressure

M REDOLFI; N BLIN-SIMIAND; X DUTEN; S PASQUIERS; K HASSOUNI

doi:10.1088/2058-6272/ab01c7

Plasma Science and Technology > 2019 > 21(5): 55503-055503. > DOI: 10.1088/2058-6272/ab01c7

M REDOLFI, N BLIN-SIMIAND, X DUTEN, S PASQUIERS, K HASSOUNI. Naphthalene oxidation by different non-thermal electrical discharges at atmospheric pressure[J]. Plasma Science and Technology, 2019, 21(5): 55503-055503. DOI: 10.1088/2058-6272/ab01c7

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Naphthalene oxidation by different non-thermal electrical discharges at atmospheric pressure

¹ LSPM, CNRS-UPR3407, Université Paris 13 Sorbonne Paris Cité, 99 Avenue J. B. Clément, F-93430, Villetaneuse, France
² Laboratoire de Physique des Gaz et des Plasmas, CNRS-UMR8578, Université Paris-Sud, Bat. 210, F-91405, Orsay Cedex, France

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Received Date: August 23, 2018

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Abstract

Gaseous naphthalene has been removed by air plasma generated by pulsed corona discharges at 100°C (LSPM) and dielectric barrier discharges (DBD) up to 250 °C (LPGP) in different reactors geometries. Naphthalene has been chosen as one of unburned hydrocarbon present in exhaust gas engine during the cold start of vehicles. The comparison between the different discharge geometries has been possible using the specific input energy (SIE) as relevant parameter for pollutant removal process control considering the differences in the electrical characteristics and the differences of gas flow. The best naphthalene degradation is obtained in the wire-to cylinder (WTC) corona discharge and the stem-to-cylinder DBD with an energy cost β respectively of 10 and 20 J L ^-1. The main by-products issues of the naphthalene oxidation are CO₂ and CO reaching 45% in Multi-Pin-to-Plan corona discharge. We detected polyaromatic hydrocarbons in the gas phase (few ppm) and in the solid phase deposited in the reactors. The introduction of water in the discharges promotes the naphthalene degradation by OH-atom, which has better oxidising power than O-atom in dry air.
- corona discharges,
- DBD,
- naphtalene,
- engine emissions

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Naphthalene oxidation by different non-thermal electrical discharges at atmospheric pressure