Yield of Ozone, Nitrite Nitrogen and Hydrogen Peroxide Versus Discharge Parameter Using APPJ Under Water

CHEN Bingyan (陈秉岩); ZHU Changping (朱昌平); FEI Juntao (费峻涛); HE Xiang (何湘); YIN Cheng (殷澄); WANG Yuan (王媛); GAO Ying (高莹); JIANG Yongfeng (蒋永锋); WEN Wen (文文); CHEN Longwei (陈龙威)

doi:10.1088/1009-0630/18/3/11

Plasma Science and Technology > 2016 > 18(3): 278-286. > DOI: 10.1088/1009-0630/18/3/11

CHEN Bingyan (陈秉岩), ZHU Changping (朱昌平), FEI Juntao (费峻涛), HE Xiang (何湘), YIN Cheng (殷澄), WANG Yuan (王媛), GAO Ying (高莹), JIANG Yongfeng (蒋永锋), WEN Wen (文文), CHEN Longwei (陈龙威). Yield of Ozone, Nitrite Nitrogen and Hydrogen Peroxide Versus Discharge Parameter Using APPJ Under Water[J]. Plasma Science and Technology, 2016, 18(3): 278-286. DOI: 10.1088/1009-0630/18/3/11

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Yield of Ozone, Nitrite Nitrogen and Hydrogen Peroxide Versus Discharge Parameter Using APPJ Under Water

1Department of Mathematics and Physics, Hohai University, Changzhou 213022, China 2Jiangsu Province Key Laboratory of Environmental Engineering, Nanjing 210036, China 3Hohai University Nantong Institute of Marine and Offshore Engineering, Nantong 226300, China 4College of Energy and Electrical Engineering, Hohai University, Nanjing 210098, China 5College of Internet of Things, Hohai University, Changzhou 213022, China 6College of Mechanical and Electrical Engineering, Hohai University, Changzhou 213022, China 7Institute of Plasma Physics, Chinese Academy of Sciences, Hefei 230031, China

Funds: supported by National Natural Science Foundation of China (Nos. 11274092, 11404092, 61401146), the Nantong Science and Technology Project, Nantong, China (No. BK2014024), the Open Project of Jiangsu Province Key Laboratory of Environmental Engineering,Nanjing, China (No. KF2014001), and the Fundamental Research Funds for the Central Universities of China (No. 2014B11414)

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Received Date: September 07, 2015

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Abstract

Abstract

Discharge plasma in and in contact with water can be accompanied with ultraviolet radiation and electron impact, thus can generate hydroxyl radicals, ozone, nitrite nitrogen and hydrogen peroxide. In this paper, a non-equilibrium plasma processing system was established by means of an atmospheric pressure plasma jet immersed in water. The hydroxyl intensities and discharge energy waveforms were tested. The results show that the positive and negative discharge energy peaks were asymmetric, where the positive discharge energy peak was greater than the negative one. Meanwhile, the yield of ozone and nitrite nitrogen was enhanced with the increase of both the treatment time and the discharge energy. Moreover, the pH value of treated water was reduced rapidly and maintained at a lower level. The residual concentration of hydrogen peroxide in APPJ treated water was kept at a low level. Additionally, both the efficiency energy ratio of the yield of ozone and nitrite nitrogen and that of the removal of p-nitrophenol increased as a function of discharge energy and discharge voltage. The experimental results were fully analyzed and the chemical reaction equations and the physical processes of discharges in water were given.
- atmospheric pressure plasma jet,
- underwater discharge,
- ozone, nitrite nitrogen

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References

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